Andy Tanjaroon Ly , Benjamin Cohen-Stead , Sohan Malkaruge Costa , and Steven Johnston
Phys. Rev. B 108, 184501 – Published 1 November, 2023
Publication year: 2023

Theoretical studies suggest that Su-Schrieffer-Heeger-like electron-phonon (𝑒-ph) interactions can mediate high-temperature bipolaronic superconductivity that is robust against repulsive electron-electron interactions. Here we present a comparative analysis of the pairing and competing charge/bond correlations in the two-dimensional Holstein and optical Su-Schrieffer-Heeger (SSH) models using numerically exact determinant quantum Monte Carlo. We find that the SSH interactions support light bipolarons and strong superconducting correlations out to relatively large values of the 𝑒-ph coupling 𝜆 and densities near half-filling, while the Holstein interaction does not due to the formation of heavy bipolarons and competing charge-density-wave order. We further find that the Holstein and SSH models have comparable pairing correlations in the weak coupling limit for carrier concentrations ⟨𝑛⟩≪1, where competing orders and polaronic effects are absent. These results support the proposal that SSH (bi)polarons can support superconductivity to larger values of 𝜆 in comparison to the Holstein polaron, but that the resulting 𝑇c gains are small in the weak coupling limit. We also find that the SSH model’s pairing correlations are suppressed after including a weak on-site Hubbard repulsion. These results have important implications for identifying and engineering bipolaronic superconductivity.